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Additional resources for Advances in Chemical Physics: The Application of Wave Mechanical Methods to the Study of Molecular Properties, Volume 8
Schematic absorption spectra of one-dimensional mixed crystals, m = 6, with inverted bands, for various trap depths 6. The intensities are adjusted to give equal values in the third transition, except in the top (pure crystal) spectrum. Hatching indicates very intense absorption. the spectral lines more dense, until in very low concentrations we expect a quasi-continuum of absorption lines. In a sufficiently thick crystal we might expect to find absorption with onset roughly at a frequency for the lowest level of the band and running with varying intensity to a maximum at the top of the band.
The dotted lines show the values given by the limiting formulae. I Fig. 2. The energy levels as a function of trap depth d for the onedimensional mixed crystal with guest concentration +. The manifold shown belongs to Y = 0. The dotted curves are plots of the shallowtrap (left-hand) and deep-trap (right-hand) limiting approximations. In the limit of large 6 the system of m molecules goes into independent sub-systems, one of them the guest molecule alone and the other the residual host consisting of groups of m - 1 host molecules separated from other groups by the guests.
Spectr. 12, 98 (1964). Naiman, C. , and Linz, Arthur, Proceedings of the Symposium on Optical Masers, Polytechnic Press, Brooklyn, 1963,p. 369. , J . Phys. Japan 18, 1719 (1963). Poole, C. , Jr.. J . Chem. Phys. 39, 3445 (1963). , and Rice, S. , J . Chew. Phys. 40, 2018 (1964). Sturge, M. , Phys. Rev. 130, 639 (1963). ,and Shulman, R. , Phys. Rev. 130, 517 (1963). , J . Phys. Soc. Japan 18, 1391 (1963). , and McClure, D. , J . Appl. Phys. SuppZ. 33,347 (1962). , J. Chem. Phys. 36, 2117 (1962). , and Dillon, J.
Advances in Chemical Physics: The Application of Wave Mechanical Methods to the Study of Molecular Properties, Volume 8